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Investigating Apparent Deviations from Darcy’s Law in Heterogeneous Rocks : Insights from Neutron Imaging

Vieira Lima, Fernando LU ; Hall, Stephen A. LU ; Engqvist, Jonas LU orcid ; Tudisco, Erika LU orcid ; Woracek, Robin ; Athanasopoulos, Stefanos LU and Vestin, Philip LU (2025) In Transport in Porous Media 152(7).
Abstract

Darcy’s law provides a fundamental framework for understanding fluid flow through porous media. However, deviations from its linear superficial velocity-hydraulic gradient (v-i) relationship have been widely reported, at high and low flow rates. While previous studies have attributed the low flow rate deviations to factors such as fluid properties, boundary effects, and experimental artifacts, the role of material heterogeneity has received less attention. This study employs neutron imaging to investigate how rock heterogeneity influences macroscopically observed flow behavior. Volume-controlled percolation tests were conducted on Idaho Gray sandstone cores under near-single-phase conditions using heavy water (D2O) and normal... (More)

Darcy’s law provides a fundamental framework for understanding fluid flow through porous media. However, deviations from its linear superficial velocity-hydraulic gradient (v-i) relationship have been widely reported, at high and low flow rates. While previous studies have attributed the low flow rate deviations to factors such as fluid properties, boundary effects, and experimental artifacts, the role of material heterogeneity has received less attention. This study employs neutron imaging to investigate how rock heterogeneity influences macroscopically observed flow behavior. Volume-controlled percolation tests were conducted on Idaho Gray sandstone cores under near-single-phase conditions using heavy water (D2O) and normal water (H2O) across a wide range of flow rates. Bulk measurements (pore pressure at the sample boundaries and the controlled injection flow rate) revealed a decline in hydraulic conductivity at lower injection rates. Through a novel method for interpreting the breakthrough curves (BTC) derived from the neutron imaging data, we are able to quantify the volume of pores active in the flow during each test. The neutron radiography imaging acquired during the flow tests revealed that flow paths were strongly influenced by the rock’s heterogeneous pore structure, with higher flow rates promoting more uniform front propagation. This suggests greater pore space access at higher injection rates and implies the presence of threshold pressure gradients needed to access different parts of the pore network. The BTC analysis from neutron image shows a decrease in the volume of pores active in the flow (effective porosity) with decreasing injection rates, aligning with the observed reduction in hydraulic conductivity. By linking nonlinearity in vi-curves to variations in effective porosity, this study highlights the critical role of heterogeneity in controlling the fluid flow behavior. These findings underscore the importance of understanding the role of spatial variability in porous media when interpreting macroscopic (bulk) permeability measurements, especially when interpreting apparent deviations from Darcy’s law.

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author
; ; ; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
Breakthrough curves, In situ neutron imaging, Rock heterogeneity, Rock hydraulic conductivity
in
Transport in Porous Media
volume
152
issue
7
article number
46
publisher
Springer
external identifiers
  • scopus:105007755291
ISSN
0169-3913
DOI
10.1007/s11242-025-02185-1
language
English
LU publication?
yes
additional info
Publisher Copyright: © The Author(s) 2025.
id
9485fec3-5d4d-460e-8253-53319f1ca83a
date added to LUP
2025-06-23 08:22:28
date last changed
2025-06-26 16:20:29
@article{9485fec3-5d4d-460e-8253-53319f1ca83a,
  abstract     = {{<p>Darcy’s law provides a fundamental framework for understanding fluid flow through porous media. However, deviations from its linear superficial velocity-hydraulic gradient (v-i) relationship have been widely reported, at high and low flow rates. While previous studies have attributed the low flow rate deviations to factors such as fluid properties, boundary effects, and experimental artifacts, the role of material heterogeneity has received less attention. This study employs neutron imaging to investigate how rock heterogeneity influences macroscopically observed flow behavior. Volume-controlled percolation tests were conducted on Idaho Gray sandstone cores under near-single-phase conditions using heavy water (D<sub>2</sub>O) and normal water (H<sub>2</sub>O) across a wide range of flow rates. Bulk measurements (pore pressure at the sample boundaries and the controlled injection flow rate) revealed a decline in hydraulic conductivity at lower injection rates. Through a novel method for interpreting the breakthrough curves (BTC) derived from the neutron imaging data, we are able to quantify the volume of pores active in the flow during each test. The neutron radiography imaging acquired during the flow tests revealed that flow paths were strongly influenced by the rock’s heterogeneous pore structure, with higher flow rates promoting more uniform front propagation. This suggests greater pore space access at higher injection rates and implies the presence of threshold pressure gradients needed to access different parts of the pore network. The BTC analysis from neutron image shows a decrease in the volume of pores active in the flow (effective porosity) with decreasing injection rates, aligning with the observed reduction in hydraulic conductivity. By linking nonlinearity in vi-curves to variations in effective porosity, this study highlights the critical role of heterogeneity in controlling the fluid flow behavior. These findings underscore the importance of understanding the role of spatial variability in porous media when interpreting macroscopic (bulk) permeability measurements, especially when interpreting apparent deviations from Darcy’s law.</p>}},
  author       = {{Vieira Lima, Fernando and Hall, Stephen A. and Engqvist, Jonas and Tudisco, Erika and Woracek, Robin and Athanasopoulos, Stefanos and Vestin, Philip}},
  issn         = {{0169-3913}},
  keywords     = {{Breakthrough curves; In situ neutron imaging; Rock heterogeneity; Rock hydraulic conductivity}},
  language     = {{eng}},
  number       = {{7}},
  publisher    = {{Springer}},
  series       = {{Transport in Porous Media}},
  title        = {{Investigating Apparent Deviations from Darcy’s Law in Heterogeneous Rocks : Insights from Neutron Imaging}},
  url          = {{http://dx.doi.org/10.1007/s11242-025-02185-1}},
  doi          = {{10.1007/s11242-025-02185-1}},
  volume       = {{152}},
  year         = {{2025}},
}