Skip to main content

Lund University Publications

LUND UNIVERSITY LIBRARIES

Two-Phase Fluid Dynamics in Proton Exchange Membrane Fuel Cells : Counter-Flow Liquid Inlets and Gas Outlets at the Electrolyte-Cathode Interface

Yang, Danan LU ; Beale, Steven B. ; Garg, Himani LU orcid and Andersson, Martin LU (2024) In Journal of the Electrochemical Society 171(10).
Abstract

Understanding the counter-flow of liquid inlet and gas outlet at the interface between the electrolyte and cathode gas diffusion layer (GDL) is crucial for water management in proton exchange membrane fuel cells. Existing studies typically overlook air outlets and assume a fixed liquid inlet direction. This study uses a volume of fluid method to model two-phase interactions in a T-shaped GDL and gas channel (GC) assembly, with GDL geometry derived from nano-computer tomography. Considering potential electrode deformations, such as local cracks and blockages, this research investigates the impact of the size and shape of liquid invasion on the liquid-gas behavior in the cathode GDL and GC using five liquid injection configurations.... (More)

Understanding the counter-flow of liquid inlet and gas outlet at the interface between the electrolyte and cathode gas diffusion layer (GDL) is crucial for water management in proton exchange membrane fuel cells. Existing studies typically overlook air outlets and assume a fixed liquid inlet direction. This study uses a volume of fluid method to model two-phase interactions in a T-shaped GDL and gas channel (GC) assembly, with GDL geometry derived from nano-computer tomography. Considering potential electrode deformations, such as local cracks and blockages, this research investigates the impact of the size and shape of liquid invasion on the liquid-gas behavior in the cathode GDL and GC using five liquid injection configurations. Simulations also incorporate GDL gas outlets, integrating them with a tailored liquid inlet setup. Results show that the injection site and configuration significantly affect water behavior in the GDL, affecting saturation, stabilization, and breakthrough, followed by drainage in the GCs. Comparisons of simulations with and without air outflow show distinct counter-flow interactions, highlighting variations in water distribution and discrepancies in two-phase transport across the GCs.

(Less)
Please use this url to cite or link to this publication:
author
; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
gas channel, gas diffusion layer, liquid inlet/gas outlet, PEMFC, volume of fluid method, water saturation
in
Journal of the Electrochemical Society
volume
171
issue
10
article number
104501
pages
15 pages
publisher
Electrochemical Society
external identifiers
  • scopus:85206239650
ISSN
0013-4651
DOI
10.1149/1945-7111/ad7d3d
language
English
LU publication?
yes
additional info
Publisher Copyright: © 2024 The Author(s). Published on behalf of The Electrochemical Society by IOP Publishing Limited.
id
f2a83e4d-919b-4fe7-abdd-dafbe85f74ae
date added to LUP
2024-10-24 16:14:37
date last changed
2024-10-28 10:28:40
@article{f2a83e4d-919b-4fe7-abdd-dafbe85f74ae,
  abstract     = {{<p>Understanding the counter-flow of liquid inlet and gas outlet at the interface between the electrolyte and cathode gas diffusion layer (GDL) is crucial for water management in proton exchange membrane fuel cells. Existing studies typically overlook air outlets and assume a fixed liquid inlet direction. This study uses a volume of fluid method to model two-phase interactions in a T-shaped GDL and gas channel (GC) assembly, with GDL geometry derived from nano-computer tomography. Considering potential electrode deformations, such as local cracks and blockages, this research investigates the impact of the size and shape of liquid invasion on the liquid-gas behavior in the cathode GDL and GC using five liquid injection configurations. Simulations also incorporate GDL gas outlets, integrating them with a tailored liquid inlet setup. Results show that the injection site and configuration significantly affect water behavior in the GDL, affecting saturation, stabilization, and breakthrough, followed by drainage in the GCs. Comparisons of simulations with and without air outflow show distinct counter-flow interactions, highlighting variations in water distribution and discrepancies in two-phase transport across the GCs.</p>}},
  author       = {{Yang, Danan and Beale, Steven B. and Garg, Himani and Andersson, Martin}},
  issn         = {{0013-4651}},
  keywords     = {{gas channel; gas diffusion layer; liquid inlet/gas outlet; PEMFC; volume of fluid method; water saturation}},
  language     = {{eng}},
  month        = {{10}},
  number       = {{10}},
  publisher    = {{Electrochemical Society}},
  series       = {{Journal of the Electrochemical Society}},
  title        = {{Two-Phase Fluid Dynamics in Proton Exchange Membrane Fuel Cells : Counter-Flow Liquid Inlets and Gas Outlets at the Electrolyte-Cathode Interface}},
  url          = {{http://dx.doi.org/10.1149/1945-7111/ad7d3d}},
  doi          = {{10.1149/1945-7111/ad7d3d}},
  volume       = {{171}},
  year         = {{2024}},
}