Breakdown of the Structure–Function Relationship on a Polycrystalline Pd Catalyst Surface Illustrated by Dynamic CO Oxidation
(2026) In ACS Catalysis 16(8). p.7281-7288- Abstract
Real catalysts consisting of nanoparticles host many nanofacets. Each nanofacet changes its structure and function in response to its local environment but is also affected by neighboring nanofacets. Time-resolved operando experiments close to realistic conditions at polycrystals mimicking real catalyst particles are unfortunately challenging but could be highly rewarding. Here, we demonstrate how such studies can be performed with time-resolved ambient pressure X-ray photoelectron spectroscopy in the millibar regime and how the local surface composition/adsorbates and gas composition can be measured simultaneously for grains on a Pd polycrystal. For the CO oxidation reaction, we demonstrate how the ignition and extinction are... (More)
Real catalysts consisting of nanoparticles host many nanofacets. Each nanofacet changes its structure and function in response to its local environment but is also affected by neighboring nanofacets. Time-resolved operando experiments close to realistic conditions at polycrystals mimicking real catalyst particles are unfortunately challenging but could be highly rewarding. Here, we demonstrate how such studies can be performed with time-resolved ambient pressure X-ray photoelectron spectroscopy in the millibar regime and how the local surface composition/adsorbates and gas composition can be measured simultaneously for grains on a Pd polycrystal. For the CO oxidation reaction, we demonstrate how the ignition and extinction are gas-phase-driven and grain-independent, while the surface structure near the extinction point is highly grain-dependent.
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- author
- Prumbs, Julia
LU
; Küst, Ulrike
LU
; Gericke, Sabrina M.
LU
; Rämisch, Lisa
LU
; Scardamaglia, Mattia
LU
; Temperton, Robert
LU
; Shavorskiy, Andrey
LU
; Zetterberg, Johan
LU
and Knudsen, Jan
LU
- organization
-
- MAX IV, Technical infrastructure
- Lund Laser Centre, LLC
- LTH Profile Area: Photon Science and Technology
- LU Profile Area: Light and Materials
- Synchrotron Radiation Research
- Combustion Physics
- MAX IV Laboratory
- MAX IV, Science division
- LTH Profile Area: The Energy Transition
- LTH Profile Area: Nanoscience and Semiconductor Technology
- NanoLund: Centre for Nanoscience
- publishing date
- 2026-04
- type
- Contribution to journal
- publication status
- published
- subject
- keywords
- APXPS, CO oxidation, extinction, FT-APXPS, ignition, palladium, polycrystals, time-resolved
- in
- ACS Catalysis
- volume
- 16
- issue
- 8
- pages
- 8 pages
- publisher
- The American Chemical Society (ACS)
- external identifiers
-
- scopus:105036416890
- ISSN
- 2155-5435
- DOI
- 10.1021/acscatal.5c08153
- language
- English
- LU publication?
- yes
- id
- 89144309-3595-4a41-b3a3-a19d2c68dbd7
- date added to LUP
- 2026-05-21 11:47:24
- date last changed
- 2026-05-26 08:03:09
@article{89144309-3595-4a41-b3a3-a19d2c68dbd7,
abstract = {{<p>Real catalysts consisting of nanoparticles host many nanofacets. Each nanofacet changes its structure and function in response to its local environment but is also affected by neighboring nanofacets. Time-resolved operando experiments close to realistic conditions at polycrystals mimicking real catalyst particles are unfortunately challenging but could be highly rewarding. Here, we demonstrate how such studies can be performed with time-resolved ambient pressure X-ray photoelectron spectroscopy in the millibar regime and how the local surface composition/adsorbates and gas composition can be measured simultaneously for grains on a Pd polycrystal. For the CO oxidation reaction, we demonstrate how the ignition and extinction are gas-phase-driven and grain-independent, while the surface structure near the extinction point is highly grain-dependent.</p>}},
author = {{Prumbs, Julia and Küst, Ulrike and Gericke, Sabrina M. and Rämisch, Lisa and Scardamaglia, Mattia and Temperton, Robert and Shavorskiy, Andrey and Zetterberg, Johan and Knudsen, Jan}},
issn = {{2155-5435}},
keywords = {{APXPS; CO oxidation; extinction; FT-APXPS; ignition; palladium; polycrystals; time-resolved}},
language = {{eng}},
number = {{8}},
pages = {{7281--7288}},
publisher = {{The American Chemical Society (ACS)}},
series = {{ACS Catalysis}},
title = {{Breakdown of the Structure–Function Relationship on a Polycrystalline Pd Catalyst Surface Illustrated by Dynamic CO Oxidation}},
url = {{http://dx.doi.org/10.1021/acscatal.5c08153}},
doi = {{10.1021/acscatal.5c08153}},
volume = {{16}},
year = {{2026}},
}