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HIPPIE : a new platform for ambient-pressure X-ray photoelectron spectroscopy at the MAX IV Laboratory

Zhu, Suyun LU ; Scardamaglia, Mattia LU ; Kundsen, Jan LU ; Sankari, Rami LU ; Tarawneh, Hamed LU ; Temperton, Robert LU ; Pickworth, Louisa LU ; Cavalca, Filippo LU ; Wang, Chunlei and Tissot, Héloïse , et al. (2021) In Journal of Synchrotron Radiation 28. p.624-636
Abstract

HIPPIE is a soft X-ray beamline on the 3 GeV electron storage ring of the MAX IV Laboratory, equipped with a novel ambient-pressure X-ray photoelectron spectroscopy (APXPS) instrument. The endstation is dedicated to performing in situ and operando X-ray photoelectron spectroscopy experiments in the presence of a controlled gaseous atmosphere at pressures up to 30 mbar [1 mbar = 100 Pa] as well as under ultra-high-vacuum conditions. The photon energy range is 250 to 2200 eV in planar polarization and with photon fluxes >1012 photons s-1 (500 mA ring current) at a resolving power of greater than 10000 and up to a maximum of 32000. The endstation currently provides two sample environments: a catalysis cell and an electrochemical/liquid... (More)

HIPPIE is a soft X-ray beamline on the 3 GeV electron storage ring of the MAX IV Laboratory, equipped with a novel ambient-pressure X-ray photoelectron spectroscopy (APXPS) instrument. The endstation is dedicated to performing in situ and operando X-ray photoelectron spectroscopy experiments in the presence of a controlled gaseous atmosphere at pressures up to 30 mbar [1 mbar = 100 Pa] as well as under ultra-high-vacuum conditions. The photon energy range is 250 to 2200 eV in planar polarization and with photon fluxes >1012 photons s-1 (500 mA ring current) at a resolving power of greater than 10000 and up to a maximum of 32000. The endstation currently provides two sample environments: a catalysis cell and an electrochemical/liquid cell. The former allows APXPS measurements of solid samples in the presence of a gaseous atmosphere (with a mixture of up to eight gases and a vapour of a liquid) and simultaneous analysis of the inlet/outlet gas composition by online mass spectrometry. The latter is a more versatile setup primarily designed for APXPS at the solid-liquid (dip-and-pull setup) or liquid-gas (liquid microjet) interfaces under full electrochemical control, and it can also be used as an open port for ad hoc-designed non-standard APXPS experiments with different sample environments. The catalysis cell can be further equipped with an IR reflection-absorption spectrometer, allowing for simultaneous APXPS and IR spectroscopy of the samples. The endstation is set up to easily accommodate further sample environments.

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organization
publishing date
type
Contribution to journal
publication status
published
subject
keywords
APXPS, beamline, catalysis, in situ, IR, operando, synchrotron
in
Journal of Synchrotron Radiation
volume
28
pages
13 pages
publisher
International Union of Crystallography
external identifiers
  • scopus:85102226267
  • pmid:33650575
ISSN
1600-5775
DOI
10.1107/S160057752100103X
language
English
LU publication?
yes
id
8c4dfc33-54cd-4235-ac41-fadfe169a884
date added to LUP
2021-03-24 14:23:18
date last changed
2024-06-27 10:53:02
@article{8c4dfc33-54cd-4235-ac41-fadfe169a884,
  abstract     = {{<p>HIPPIE is a soft X-ray beamline on the 3 GeV electron storage ring of the MAX IV Laboratory, equipped with a novel ambient-pressure X-ray photoelectron spectroscopy (APXPS) instrument. The endstation is dedicated to performing in situ and operando X-ray photoelectron spectroscopy experiments in the presence of a controlled gaseous atmosphere at pressures up to 30 mbar [1 mbar = 100 Pa] as well as under ultra-high-vacuum conditions. The photon energy range is 250 to 2200 eV in planar polarization and with photon fluxes &gt;1012 photons s-1 (500 mA ring current) at a resolving power of greater than 10000 and up to a maximum of 32000. The endstation currently provides two sample environments: a catalysis cell and an electrochemical/liquid cell. The former allows APXPS measurements of solid samples in the presence of a gaseous atmosphere (with a mixture of up to eight gases and a vapour of a liquid) and simultaneous analysis of the inlet/outlet gas composition by online mass spectrometry. The latter is a more versatile setup primarily designed for APXPS at the solid-liquid (dip-and-pull setup) or liquid-gas (liquid microjet) interfaces under full electrochemical control, and it can also be used as an open port for ad hoc-designed non-standard APXPS experiments with different sample environments. The catalysis cell can be further equipped with an IR reflection-absorption spectrometer, allowing for simultaneous APXPS and IR spectroscopy of the samples. The endstation is set up to easily accommodate further sample environments.</p>}},
  author       = {{Zhu, Suyun and Scardamaglia, Mattia and Kundsen, Jan and Sankari, Rami and Tarawneh, Hamed and Temperton, Robert and Pickworth, Louisa and Cavalca, Filippo and Wang, Chunlei and Tissot, Héloïse and Weissenrieder, Jonas and Hagman, Benjamin and Gustafson, Johan and Kaya, Sarp and Lindgren, Fredrik and Källquist, Ida and Maibach, Julia and Hahlin, Maria and Boix, Virginia and Gallo, Tamires and Rehman, Foqia and D'Acunto, Giulio and Schnadt, Joachim and Shavorskiy, Andrey}},
  issn         = {{1600-5775}},
  keywords     = {{APXPS; beamline; catalysis; in situ; IR; operando; synchrotron}},
  language     = {{eng}},
  pages        = {{624--636}},
  publisher    = {{International Union of Crystallography}},
  series       = {{Journal of Synchrotron Radiation}},
  title        = {{HIPPIE : a new platform for ambient-pressure X-ray photoelectron spectroscopy at the MAX IV Laboratory}},
  url          = {{http://dx.doi.org/10.1107/S160057752100103X}},
  doi          = {{10.1107/S160057752100103X}},
  volume       = {{28}},
  year         = {{2021}},
}