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2D electron gas formation on InAs wurtzite nanosheet surfaces

Benter, S. LU ; Bianchi, M. ; Pan, D. ; Zhao, J. ; Xu, H. Q. LU ; Timm, R. LU orcid ; Hofmann, Ph and Mikkelsen, A. LU (2024) In Applied Physics Letters 124(15).
Abstract

The two-dimensional electron gas (2DEG) that forms on a semiconductor surface can be used to explore a variety of phenomena in quantum physics and plays an important role in nanoscale electronics, such as transistors. Controlling its formation is, thus, relevant. Using angle-resolved photoemission spectroscopy (ARPES) and accumulating the signal over many nanocrystals, we find that on clean InAs nanosheets with non-polar surfaces and wurtzite (WZ) crystal structures, a 2DEG can be observed at the Γ-point. We suggest that the step morphology on the WZ InAs specimens facilitates the appearance of the electron gas, since previous studies on InAs nanowire surfaces with the same crystal facet and a similar defect density did not exhibit a... (More)

The two-dimensional electron gas (2DEG) that forms on a semiconductor surface can be used to explore a variety of phenomena in quantum physics and plays an important role in nanoscale electronics, such as transistors. Controlling its formation is, thus, relevant. Using angle-resolved photoemission spectroscopy (ARPES) and accumulating the signal over many nanocrystals, we find that on clean InAs nanosheets with non-polar surfaces and wurtzite (WZ) crystal structures, a 2DEG can be observed at the Γ-point. We suggest that the step morphology on the WZ InAs specimens facilitates the appearance of the electron gas, since previous studies on InAs nanowire surfaces with the same crystal facet and a similar defect density did not exhibit a 2DEG. Subsequently, bismuth deposition leads to the disappearance of the 2DEG as well as a shift of the valence band. This is in contrast to previous observations on InAs surfaces, in which metal deposition would lead to the formation of a 2DEG. The control of the 2DEG with the addition of Bi atoms is relevant for applications of InAs nanosheets in quantum technologies. This study also illustrates that ARPES accumulated over several 2D materials oriented randomly around their normal axis can provide valuable information on their band structure with a fast turnover and low irradiation.

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author
; ; ; ; ; ; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Applied Physics Letters
volume
124
issue
15
article number
153104
publisher
American Institute of Physics (AIP)
external identifiers
  • scopus:85190545635
ISSN
0003-6951
DOI
10.1063/5.0200217
language
English
LU publication?
yes
id
bd72369e-fbda-48ab-af3e-1ab9700314c0
date added to LUP
2024-05-06 14:12:09
date last changed
2024-05-06 14:13:26
@article{bd72369e-fbda-48ab-af3e-1ab9700314c0,
  abstract     = {{<p>The two-dimensional electron gas (2DEG) that forms on a semiconductor surface can be used to explore a variety of phenomena in quantum physics and plays an important role in nanoscale electronics, such as transistors. Controlling its formation is, thus, relevant. Using angle-resolved photoemission spectroscopy (ARPES) and accumulating the signal over many nanocrystals, we find that on clean InAs nanosheets with non-polar surfaces and wurtzite (WZ) crystal structures, a 2DEG can be observed at the Γ-point. We suggest that the step morphology on the WZ InAs specimens facilitates the appearance of the electron gas, since previous studies on InAs nanowire surfaces with the same crystal facet and a similar defect density did not exhibit a 2DEG. Subsequently, bismuth deposition leads to the disappearance of the 2DEG as well as a shift of the valence band. This is in contrast to previous observations on InAs surfaces, in which metal deposition would lead to the formation of a 2DEG. The control of the 2DEG with the addition of Bi atoms is relevant for applications of InAs nanosheets in quantum technologies. This study also illustrates that ARPES accumulated over several 2D materials oriented randomly around their normal axis can provide valuable information on their band structure with a fast turnover and low irradiation.</p>}},
  author       = {{Benter, S. and Bianchi, M. and Pan, D. and Zhao, J. and Xu, H. Q. and Timm, R. and Hofmann, Ph and Mikkelsen, A.}},
  issn         = {{0003-6951}},
  language     = {{eng}},
  month        = {{04}},
  number       = {{15}},
  publisher    = {{American Institute of Physics (AIP)}},
  series       = {{Applied Physics Letters}},
  title        = {{2D electron gas formation on InAs wurtzite nanosheet surfaces}},
  url          = {{http://dx.doi.org/10.1063/5.0200217}},
  doi          = {{10.1063/5.0200217}},
  volume       = {{124}},
  year         = {{2024}},
}