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Thin reaction zones in constant-density turbulent flows at low Damköhler numbers : Theory and simulations

Sabelnikov, V. A. ; Yu, R. LU and Lipatnikov, A. N. (2019) In Physics of Fluids 31(5).
Abstract


Propagation of a single-reaction wave in a constant-density turbulent flow is studied by considering reaction rates that depend on the reaction progress variable c in a highly nonlinear manner. Analysis of Direct Numerical Simulation (DNS) data obtained recently from 26 reaction waves characterized by low Damköhler (0.01 < Da < 1) and high Karlovitz (6.5 < Ka < 587) numbers reveals the following trends. First, the ratio of consumption velocity U
T
to rms turbulent velocity u′ scales as square root of Da in line with Damköhler's... (More)


Propagation of a single-reaction wave in a constant-density turbulent flow is studied by considering reaction rates that depend on the reaction progress variable c in a highly nonlinear manner. Analysis of Direct Numerical Simulation (DNS) data obtained recently from 26 reaction waves characterized by low Damköhler (0.01 < Da < 1) and high Karlovitz (6.5 < Ka < 587) numbers reveals the following trends. First, the ratio of consumption velocity U
T
to rms turbulent velocity u′ scales as square root of Da in line with Damköhler's classical hypothesis. Second, the ratio of fully developed turbulent wave thickness to an integral length scale of turbulence decreases with increasing Da and tends to scale with inverse square root of Da, in line with the same hypothesis. Third, contrary to the widely accepted concept of distributed reaction zones, reaction-zone broadening is quite moderate even at Da = 0.01 and Ka = 587. Fourth, contrary to the same concept, U
T
/u′ is mainly controlled by the reaction-surface area. Fifth, U
T
/u′ does not vary with the laminar-reaction-zone thickness, provided that Da is constant. To explain the totality of these DNS results, a new theory is developed by (i) exploring the propagation of a molecular mixing layer attached to an infinitely thin reaction sheet in a highly turbulent flow and (ii) hypothesizing that the area of the reaction sheet is controlled by turbulent mixing. This hypothesis is supported by order-of-magnitude estimates and results in the aforementioned Damköhler's scaling for U
T
/u′. The theory is also consistent with other aforementioned DNS results and, in particular, explains the weak influence of the laminar-reaction-zone thickness on U
T
/u′.

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author
; and
organization
publishing date
type
Contribution to journal
publication status
published
subject
in
Physics of Fluids
volume
31
issue
5
article number
055104
publisher
American Institute of Physics (AIP)
external identifiers
  • scopus:85065608638
ISSN
1070-6631
DOI
10.1063/1.5090192
language
English
LU publication?
yes
id
3664bd5b-1e75-46d0-a56a-d706585b0344
date added to LUP
2019-05-23 12:14:48
date last changed
2022-04-26 00:21:16
@article{3664bd5b-1e75-46d0-a56a-d706585b0344,
  abstract     = {{<p><br>
                                                         Propagation of a single-reaction wave in a constant-density turbulent flow is studied by considering reaction rates that depend on the reaction progress variable c in a highly nonlinear manner. Analysis of Direct Numerical Simulation (DNS) data obtained recently from 26 reaction waves characterized by low Damköhler (0.01 &lt; Da &lt; 1) and high Karlovitz (6.5 &lt; Ka &lt; 587) numbers reveals the following trends. First, the ratio of consumption velocity U                             <br>
                            <sub>T</sub><br>
                                                          to rms turbulent velocity u′ scales as square root of Da in line with Damköhler's classical hypothesis. Second, the ratio of fully developed turbulent wave thickness to an integral length scale of turbulence decreases with increasing Da and tends to scale with inverse square root of Da, in line with the same hypothesis. Third, contrary to the widely accepted concept of distributed reaction zones, reaction-zone broadening is quite moderate even at Da = 0.01 and Ka = 587. Fourth, contrary to the same concept, U                             <br>
                            <sub>T</sub><br>
                                                         /u′ is mainly controlled by the reaction-surface area. Fifth, U                             <br>
                            <sub>T</sub><br>
                                                         /u′ does not vary with the laminar-reaction-zone thickness, provided that Da is constant. To explain the totality of these DNS results, a new theory is developed by (i) exploring the propagation of a molecular mixing layer attached to an infinitely thin reaction sheet in a highly turbulent flow and (ii) hypothesizing that the area of the reaction sheet is controlled by turbulent mixing. This hypothesis is supported by order-of-magnitude estimates and results in the aforementioned Damköhler's scaling for U                             <br>
                            <sub>T</sub><br>
                                                         /u′. The theory is also consistent with other aforementioned DNS results and, in particular, explains the weak influence of the laminar-reaction-zone thickness on U                             <br>
                            <sub>T</sub><br>
                                                         /u′.                         <br>
                        </p>}},
  author       = {{Sabelnikov, V. A. and Yu, R. and Lipatnikov, A. N.}},
  issn         = {{1070-6631}},
  language     = {{eng}},
  number       = {{5}},
  publisher    = {{American Institute of Physics (AIP)}},
  series       = {{Physics of Fluids}},
  title        = {{Thin reaction zones in constant-density turbulent flows at low Damköhler numbers : Theory and simulations}},
  url          = {{http://dx.doi.org/10.1063/1.5090192}},
  doi          = {{10.1063/1.5090192}},
  volume       = {{31}},
  year         = {{2019}},
}